Search results for "Methylammonium lead halide"

showing 2 items of 2 documents

Humidity-Induced Grain Boundaries in MAPbI3 Perovskite Films

2016

Methylammonium lead halide perovskites (MAPbI3) are very sensitive to humid environments. We performed in situ scanning force microscopy and in situ X-ray diffraction measurements on MAPbI3 films to track changes in the film morphology and crystal structure upon repeated exposure to a high relative humidity environment (80%). We found that the appearance of monohydrate (MAPbI3·H2O) Bragg reflections coincided with the appearance of additional grain boundaries. Prolonging the exposure time to humidity induced more grain boundaries and steps in the MAPbI3 films, and the peak intensities of the monohydrate MAPbI3·H2O increased. The monohydrate was not stable under dry atmosphere and could be r…

Materials scienceAnalytical chemistryHumidity02 engineering and technologyCrystal structureMethylammonium lead halide010402 general chemistry021001 nanoscience & nanotechnology01 natural sciences0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsAtmospherechemistry.chemical_compoundCrystallographyHysteresisGeneral EnergychemistryGrain boundaryRelative humidityPhysical and Theoretical Chemistry0210 nano-technologyPerovskite (structure)The Journal of Physical Chemistry C
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Efficient vacuum deposited p-i-n and n-i-p perovskite solar cells employing doped charge transport layers

2016

Methylammonium lead halide perovskites have emerged as high performance photovoltaic materials. Most of these solar cells are prepared via solution-processing and record efficiencies (>20%) have been obtained employing perovskites with mixed halides and organic cations on (mesoscopic) metal oxides. Here, we demonstrate fully vacuum deposited planar perovskite solar cells by depositing methylammonium lead iodide in between intrinsic and doped organic charge transport molecules. Two configurations, one inverted with respect to the other, p-i-n and n-i-p, are prepared and optimized leading to planar solar cells without hysteresis and very high efficiencies, 16.5% and 20%, respectively. It is t…

Renewable Energy Sustainability and the EnvironmentChemistryPhotovoltaic systemDopingAnalytical chemistryHalidePerovskite solar cellNanotechnology02 engineering and technologyHybrid solar cellMethylammonium lead halide010402 general chemistry021001 nanoscience & nanotechnology01 natural sciencesPollutionPolymer solar cell0104 chemical scienceschemistry.chemical_compoundNuclear Energy and EngineeringEnvironmental Chemistry0210 nano-technologyMaterialsCèl·lules fotoelèctriquesPerovskite (structure)Energy Environ. Sci.
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